It's harder than I thought to come up with great films that weren't based on a book.. A few good ones already mentioned, like Night of the Living Dead and 28 Days Later. I'd also add:
Blood On Satan's Claw
Eye Of The Devil
The Exorcist
Witchfinder General
Rasputin The Mad Monk
Some of those are based on real-life events, if that's OK.
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